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  1. Abstract

    The export of deep water from the Arctic to the Atlantic contributes to the formation of North Atlantic Deep Water, a crucial component of global ocean circulation. Records of protactinium-231 (231Pa) and thorium-230 (230Th) in Arctic sediments can provide a measure of this export, but well-constrained sedimentary budgets of these isotopes have been difficult to achieve in the Arctic Ocean. Previous studies revealed a deficit of231Pa in central Arctic sediments, implying that some231Pa is either transported to the margins, where it may be removed in areas of higher particle flux, or exported from the Arctic via deep water advection. Here we investigate this “missing sink” of Arctic231Pa and find moderately increased231Pa deposition along Arctic margins. Nonetheless, we determine that most231Pa missing from the central basin must be lost via advection into the Nordic Seas, requiring deep water advection of 1.1 – 6.4 Sv through Fram Strait.

     
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  2. Abstract

    The flux of terrestrial material from the continents to the oceans links the lithosphere, hydrosphere, and biosphere through physical and biogeochemical processes, with important implications for Earth's climate. Quantitative estimates of terrigenous fluxes from sources such as rivers, aeolian dust, and resuspended shelf sediments are required to understand how the processes delivering terrigenous material respond to and are influenced by climate. We compile thorium‐230 normalized232Th flux records in the tropical Atlantic to provide an improved understanding of aeolian fluxes since the Last Glacial Maximum (LGM). By identifying and isolating sites dominated by aeolian terrigenous inputs, we show that there was a persistent meridional gradient in dust fluxes in the eastern equatorial Atlantic at the LGM, arguing against a large southward shift of the intertropical convergence zone during LGM boreal winter. The ratio of LGM to late‐Holocene232Th fluxes highlights a meridional difference in the magnitude of variations in dust deposition, with sites <10°N showing larger changes over time. This supports an interpretation of increased trade wind strength at the LGM, potentially combined with differential changes in soil moisture and reductions in higher altitude summer winds. Our results also highlight the persistent importance of continental margins as sources of high terrigenous flux to the open ocean. This is especially evident in the western tropical Atlantic, where study locations reveal the primary influence of the South American continent up to >700 km away, characterized by232Th fluxes approximately twice as large as aeolian‐dominated sites in the east.

     
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  3. While the Atlantic Ocean is ventilated by high-latitude deep water formation and exhibits a pole-to-pole overturning circulation, the Pacific Ocean does not. This asymmetric global overturning pattern has persisted for the past 2–3 million years, with evidence for different ventilation modes in the deeper past. In the current climate, the Atlantic-Pacific asymmetry occurs because the Atlantic is more saline, enabling deep convection. To what extent the salinity contrast between the two basins is dominated by atmospheric processes (larger net evaporation over the Atlantic) or oceanic processes (salinity transport into the Atlantic) remains an outstanding question. Numerical simulations have provided support for both mechanisms; observations of the present climate support a strong role for atmospheric processes as well as some modulation by oceanic processes. A major avenue for future work is the quantification of the various processes at play to identify which mechanisms are primary in different climate states. 
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  4. Abstract

    While substantial changes in thermohaline circulation related to deglacial climate variability are well established, the role of this circulation in Holocene climate variability remains uncertain. Here we use two dynamical proxies,231Pa/230Th ratios and mean sortable silt size (), to reconstruct Holocene bottom water circulation at the intermediate‐depth Carolina Slope. We find no substantial change in deep current speed or231Pa export at this site during the Holocene, suggesting consistent231Pa export via the Deep Western Boundary Current.shows increasing millennial‐scale variability in the middle‐late Holocene, which may reflect Labrador Sea Water contribution to current speed. We conclude that deepwater export from the North Atlantic has remained remarkably stable during the Holocene, decoupled from changing rates of specific water masses, while production of these water masses varied at millennial to centennial time scales. The persistence of the large‐scale overturning may reflect the ocean's stabilizing influence on Holocene climate.

     
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  5. Abstract

    230Th normalization is a valuable paleoceanographic tool for reconstructing high‐resolution sediment fluxes during the late Pleistocene (last ~500,000 years). As its application has expanded to ever more diverse marine environments, the nuances of230Th systematics, with regard to particle type, particle size, lateral advective/diffusive redistribution, and other processes, have emerged. We synthesized over 1000 sedimentary records of230Th from across the global ocean at two time slices, the late Holocene (0–5,000 years ago, or 0–5 ka) and the Last Glacial Maximum (18.5–23.5 ka), and investigated the spatial structure of230Th‐normalized mass fluxes. On a global scale, sedimentary mass fluxes were significantly higher during the Last Glacial Maximum (1.79–2.17 g/cm2kyr, 95% confidence) relative to the Holocene (1.48–1.68 g/cm2kyr, 95% confidence). We then examined the potential confounding influences of boundary scavenging, nepheloid layers, hydrothermal scavenging, size‐dependent sediment fractionation, and carbonate dissolution on the efficacy of230Th as a constant flux proxy. Anomalous230Th behavior is sometimes observed proximal to hydrothermal ridges and in continental margins where high particle fluxes and steep continental slopes can lead to the combined effects of boundary scavenging and nepheloid interference. Notwithstanding these limitations, we found that230Th normalization is a robust tool for determining sediment mass accumulation rates in the majority of pelagic marine settings (>1,000 m water depth).

     
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